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Beilstein J. Org. Chem. 2016, 12, 1904–1910, doi:10.3762/bjoc.12.180
Graphical Abstract
Scheme 1: Catalytic reactions of diazocarbonyl compounds with unsaturated δ-amino esters.
Figure 1: The structures of the starting compounds 1–3 and catalysts used in this study.
Scheme 2: The assumed pathway for the occurance of amides 6a–c by way of the catalytic Wolff rearrangement.
Scheme 3: The assumed mechanism for the formation of the amides 4 and 7 during oxidative cleavage of the N–H-...